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Science Paper Unveils Organic Electrolyte That Moves Ions in Solids Like a Liquid

Disc-shaped molecular ions with flexible sidechains create ordered columns that preserve liquid-like mobility in the solid state.

Overview

  • Researchers report ‘state-independent electrolytes’ that maintain high ionic conductivity across liquid, liquid-crystal and solid phases, confirmed in experiments published Dec. 18 in Science.
  • The materials use charge-delocalized, disc-like organic cations that stack into columns while long, flexible sidechains form a permeable environment for anions to move freely.
  • Conductivity follows temperature smoothly with no freeze-out on solidification, and the behavior was reproduced with several counterion types in laboratory tests.
  • The collaboration spans the Universities of Oxford, York, Leeds and Durham with partners in Portugal, Germany and the Czech Republic.
  • Potential uses include casting the electrolyte as a warm liquid for intimate electrode contact before cooling to a safe solid for batteries, sensors and electrochromic devices, as teams work to boost conductivity, add cation-conducting variants and integrate the materials into memory hardware.